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CCL 2019 30( 01) Published: 22 January 2019
Reviews
Deciphering nucleic acid modifications by chemical derivatization-mass spectrometry analysis
Meng-Dan Lan, Bi-Feng Yuan, Yu-Qi Feng
CCL 2019 Vol. 30 (01): 1-6
DOI:10.1016/j.cclet.2018.04.021
Abstract
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Chemical derivatization in combination with mass spectrometry (MS) analysis is a promising strategy for the sensitive and effective analysis of nucleic acid modifications. In this review, we summarize the recent advances for deciphering modifications in DNA and RNA by chemical derivatization-MS analysis.
Mechanochemistry in cancer cell metastasis
Di Zhang, Feng Feng, Ruping Liu, Wenjia Zhu, Li Yao
CCL 2019 Vol. 30 (01): 7-14
DOI:10.1016/j.cclet.2018.06.011
Abstract
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In this review, we introduced the mechanical factors in cancer cell metastasis, intracellular mechanical sensors and methods to measure the mechanical forces of tumor cells for evaluating the mechanochemistry in cancer metastasis.
Selectively transform lignin into value-added chemicals
Qingqing Mei, Xiaojun Shen, Huizhen Liu, Buxing Han
CCL 2019 Vol. 30 (01): 15-24
DOI:10.1016/j.cclet.2018.04.032
Abstract
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48
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Selective transformation of lignin into value-added chemicals is of strategic significance. Phenols, aldehydes, carboxylic acids, alkanes and arenes can be harvested from lignin with high selectivity under appropriate reaction condition.
Embedding pyridine units in acceptors to construct donor-acceptor conjugated polymers
Zi-Yuan Wang, Jie-Yu Wang, Jian Pei
CCL 2019 Vol. 30 (01): 25-30
DOI:10.1016/j.cclet.2018.07.006
Abstract
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Embedding pyridine units into donor-acceptor (D-A) conjugated polymer backbones results in lowered lowest unoccupied molecular orbitals (LUMOs) and improved coplanarity of polymer backbones by the non-bonding interactions, leading to high-performance semiconducting polymers.
Artificial light-harvesting systems fabricated by supramolecular host-guest interactions
Tangxin Xiao, Weiwei Zhong, Ling Zhou, Lixiang Xu, Xiao-Qiang Sun, Robert B. P. Elmes, Xiao-Yu Hu, Leyong Wang
CCL 2019 Vol. 30 (01): 31-36
DOI:10.1016/j.cclet.2018.05.034
Abstract
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46
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Recent progress on artificial light-harvesting systems fabricated by supramolecular host-guest interaction was summarized.
Water-soluble supramolecular polymers constructed by macrocycle-based host-guest interactions
Yanmei Chen, Siyu Sun, Dou Lu, Yujun Shi, Yong Yao
CCL 2019 Vol. 30 (01): 37-43
DOI:10.1016/j.cclet.2018.10.022
Abstract
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Water soluble supramolecular polymers are especially important due to their superior biocompatibility and environmental adaptation, which determined they have wide applications in various areas, such as drug delivery, self-healing, shape memory. On the other hand, macrocyclic compounds are the most used building blocks in the preparation of supramolecular polymers. Macrocycle-based supramolecular polymers, which introduce the host-guest interaction in the system, endow these polymers with interesting and smart physicalchemical properties. In this review, we summarized recent studies about supramolecular polymers in aqueous solution based on macrocyclic compounds.
Communications
Chartrenoline, a novel alkaloid isolated from a marine
Streptomyces chartreusis
NA02069
Chengli Liu, Chenglong Yang, Yingjie Zeng, Jing Shi, TD, DIF, Lingyu Li, Wei Li, Ruihua Jiao, Renxiang Tan, Huiming Ge
CCL 2019 Vol. 30 (01): 44-46
DOI:10.1016/j.cclet.2018.10.030
Abstract
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A novel alkaloid featuring a unique tetracyclic ring system was isolated from a marine actinobacterium.
Diterpenoids from the aerial parts of
Leonurus macranthus
Yunfang Zhao, Zheng Huang, Jing Sun, Daoran Pang, Xiaonan Chen, Huina Yao, Zhixiang Zhu, Jiao Zheng, Pengfei Tu, Jun Li
CCL 2019 Vol. 30 (01): 47-50
DOI:10.1016/j.cclet.2017.11.033
Abstract
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38
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One
cis
clerodane-type (
1
) and three highly oxygenated labdane-type diterpenes (
2-4
) were isolated from the aerial parts of
Leonurus macranthus
. Compound
1
represents the first example of cis clerodane-type diterpene in the plants of
Leonurus
genus.
Dimericbiscognienynes B and C: New diisoprenyl-cyclohexene-type meroterpenoid dimers from
Biscogniauxia
sp.
Huan Zhao, Meizhi Wang, Guodong Chen, Dan Hu, Enqing Li, Yibo Qu, Libing Zhou, Liangdong Guo, Xinsheng Yao, Hao Gao
CCL 2019 Vol. 30 (01): 51-54
DOI:10.1016/j.cclet.2018.05.019
Abstract
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Till now, only three diisoprenyl-cyclohexene/ane-type meroterpenoid dimers have been identified. The isolation of two new diisoprenyl-cyclohexene-type meroterpenoid dimers (dimericbiscognienynes B and C) from
Biscogniauxia
sp. 71-10-1-1 added new members to this family.
A lysosomal targeting fluorescent probe and its zinc imaging in SH-SY5Y human neuroblastoma cells
Houna Duan, Yu Ding, Chusen Huang, Weiping Zhu, Rui Wang, Yufang Xu
CCL 2019 Vol. 30 (01): 55-57
DOI:10.1016/j.cclet.2018.03.016
Abstract
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A fluorescent probe based PET mechanism was designed, and the probe could image endogenous release of Zn
2+
upon H
2
O
2
stimulation in SH-SY5Y cells.
G-quadruplex-assisted enzyme strand recycling for amplified label-free fluorescent detection of UO
2
2+
Paijin Zhu, Yiying Zhang, Shuxia Xu, Xinfeng Zhang
CCL 2019 Vol. 30 (01): 58-62
DOI:10.1016/j.cclet.2018.02.003
Abstract
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A G-quadruplex-assisted enzyme strand recycling strategy was developed for amplified label-free fluorescent detection of uranyl ion (UO
2
2+
).
A specific and selective chemiluminescent probe for Pd
2+
detection
Yuqi Gao, Yuxing Lin, Tingting Liu, Xiaomeng Zhang, Feng Xu, Pan Liu, Lupei Du, Minyong Li
CCL 2019 Vol. 30 (01): 63-66
DOI:10.1016/j.cclet.2018.03.028
Abstract
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A modified 1,2-dioxetane is reported as a chemiluminescent imaging (CLI) approach for monitoring palladium(Ⅱ).
Intracellular effects of prodrug-like wortmannin probes
Shasha Ying, Shubo Du, Jia Dong, Bi Xuan Ng, Chengwu Zhang, Lin Li, Jingyan Ge, Qing Zhu
CCL 2019 Vol. 30 (01): 67-70
DOI:10.1016/j.cclet.2018.05.030
Abstract
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A small library of wortmannin based probes was synthesized by installing a clickable handle at C11 site for bioconjugation, and secondary amine and biotin moiety at C20 site to achieve self-activation and cancer target, respectively, to facilitate the analysis of their intracellular effects.
Novel strategy of constructing fluorescent probe for MAO-B
via
cascade reaction and its application in imaging MAO-B in human astrocyte
Huihuan Qin, Lingling Li, Kun Li, Xiaoqi Yu
CCL 2019 Vol. 30 (01): 71-74
DOI:10.1016/j.cclet.2018.05.018
Abstract
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A novel strategy was developed to detect MAO-B and image MAO-B in human astrocyte by constructing coumarin via cascade reaction and intramolecular cyclization.
A water-stable lanthanide-coordination polymer with free Lewis site for fluorescent sensing of Fe
3+
Wenhe Wang, Qiang Gao, Xiaoyu Li, Jianhong Wang, Chaopeng Wang, Yinghui Zhang, Xianhe Bu
CCL 2019 Vol. 30 (01): 75-78
DOI:10.1016/j.cclet.2018.06.014
Abstract
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A Tb
3+
based coordination polymer (
NKU-115
) with free N sites was successfully constructed, featuring strong green light emission and selective quenching response toward Fe
3+
in aqueous solution.
Synthesis of AgInS
2
QDs in droplet microreactors: Online fluorescence regulating through temperature control
Haotian Ma, Liangjun Pan, Ji Wang, Li Zhang, Zhiling Zhang
CCL 2019 Vol. 30 (01): 79-82
DOI:10.1016/j.cclet.2018.04.033
Abstract
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We designed a temperature-controllable droplet microreactor with more precisely temperature control and shorter synthesis time for water-soluble AgInS
2
QDs synthesis. When reaction temperature increased from 30 ℃ to 70 ℃, QDs fluorescence peak constantly red-shifted from 590 nm to 720 nm along with enhanced fluorescence QY and intensity, we can get products with the maximum fluorescence intensity and the QY of 8.8% at 70 ℃.
Evaluation of necrosis avidity of radioiodinated 5-hydroxytryptophan and its potential applications in myocardial infarction imaging
Lin Ma, Lingqiao Cai, Qiaomei Jin, Jiajia Liang, Dongjian Zhang, Wei Liu, Yicheng Ni, Zhiqi Yin, Jian Zhang, Ke Pan
CCL 2019 Vol. 30 (01): 83-86
DOI:10.1016/j.cclet.2018.06.005
Abstract
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[
131
I]5-HTP features predominant necrosis avidity and could rapidly visualize necrotic myocardium at 3 h p.i. The necrosis avidity mechanism of [
131
I]5-HTP may be attributed to its interactions with E-DNA in the necrotic tissues.
Cancer cell detection and imaging: MRI-SERS bimodal splat-shaped Fe
3
O
4
/Au nanocomposites
Xinmei Zhao, Leyong Zeng, Narayan Hosmane, Yan Gong, Aiguo Wu
CCL 2019 Vol. 30 (01): 87-89
DOI:10.1016/j.cclet.2018.01.028
Abstract
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In this paper, a kind of splat-shaped Fe
3
O
4
/Au nanocomposites was synthesized. The magnetic resonance imaging/surface-enhanced Raman scattering (MRI/SERS) studies demonstrated that as-synthesized Fe
3
O
4
/Au nanocomposites may be a promising MRI/SERS dual probe for the tumor detection.
Effects of the ambient fine particulate matter (PM2.5) exposure on urinary metabolic profiles in rats using UPLC-Q-TOF-MS
Lin Zhang, Tengfei Xu, Zifeng Pi, Meizhu Zheng, Fengrui Song, Zhiqiang Liu
CCL 2019 Vol. 30 (01): 90-94
DOI:10.1016/j.cclet.2017.11.019
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The pathogenesis of PM2.5 was evaluated on rats in model groups using a metabonomic method by UPLC-Q-TOF-MS and 17 potential endogenous metablites were identified. The primary metabolism pathways involved pentose and glucuronate interconversions, starch and sucrose metabolism, tryptophan metabolism, tyrosine metabolism, phenylalanine metabolism, purine metabolism, acetaminophen metabolism pathway, retinol metabolism and valproic acid metabolism pathway.
A membrane separation technique for optimizing sample preparation of MALDI-TOF MS detection
Zengnan Wu, Ning Xu, Weiwei Li, Jin-Ming Lin
CCL 2019 Vol. 30 (01): 95-98
DOI:10.1016/j.cclet.2018.01.048
Abstract
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Here, we report a new method based on the combination of membrane separation technology and nanomaterial to rapid detection of peptides and protein with MALDI-TOF MS. This method shows advantages as it can inhibit the heterogeneous of sample spot and enhance the target molecular signal intensity.
Construction of on-line supercritical fluid extraction with reverse phase liquid chromatography-tandem mass spectrometry for the determination of capsaicin
Naoki Hamada, Yuki Hashi, Satoshi Yamaki, Yanli Guo, Lin Zhang, Haifang Li, Jin-Ming Lin
CCL 2019 Vol. 30 (01): 99-102
DOI:10.1016/j.cclet.2018.10.029
Abstract
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A column-switching system, composed of supercritical fluid extraction (SFE) and reverse phase liquid chromatography/mass spectrometry (RPLC/MS) was constructed for on-line extraction and reverse-phase separation of capsaicinoids in capsicum fruits.
Analysis of the binding sites with NL-101 to amino acids and peptides by HPLC/MS/MS
Lingzi Dai, Nian Guo, Yaqin Liu, Shanshan Shen, Qiufu Ge, Yuanjiang Pan
CCL 2019 Vol. 30 (01): 103-106
DOI:10.1016/j.cclet.2017.12.023
Abstract
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Collision-induced dissociation experiment demonstrated that under the same collision energy, different fragmentation pattern could help distinguish the accurate location of amino acids-NL adducts.
Dissipation behavior, residue distribution and dietary risk assessment of chlorfenapyr and clothianidin in leek using RRLC-QqQ-MS/MS technique
Xi Li, Xiaoxin Chen, Jiye Hu
CCL 2019 Vol. 30 (01): 107-110
DOI:10.1016/j.cclet.2018.02.001
Abstract
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Commercial suspension emulsion (SE) of (8% chlorfenapyr + 20% clothianidin), as a pre-registered product in China, was firstly investigated under Chinese open-field conditions. A MWCNTs-based QuEChERS method for simultaneous determination of chlorfenapyr and clothianidin in leek was established and validated through RRLC-QqQ-MS/MS.
Determination of triglycerides in human serum by near-infrared diffuse reflectance spectroscopy using silver mirror as a substrate
Shuyu Wang, Jin Zhang, Cuicui Wang, Xiaoming Yu, Wensheng Cai, Xueguang Shao
CCL 2019 Vol. 30 (01): 111-114
DOI:10.1016/j.cclet.2018.01.016
Abstract
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Quantitative determination of serum triglycerides was achieved in diffuse reflectance mode using silver mirror as the substrate to enhance the spectral features.
ATR-FTIR study of
Bacillus
sp. and
Escherichia coli
settlements on the bare and Al
2
O
3
coated ZnSe internal reflection element
Rongqiao Chen, Chune Guo, Wubo Chu, Nan Jiang, He Li
CCL 2019 Vol. 30 (01): 115-119
DOI:10.1016/j.cclet.2018.07.019
Abstract
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FTIR-ATR has been used for understanding the interaction between bacteria and surfaces in the adsorption progress.
Redox-responsive diphenylalanine aggregate mediated by cyclodextrin
Lu Zhang, Ying-Ming Zhang, Guoxing Liu, Yu Liu
CCL 2019 Vol. 30 (01): 120-122
DOI:10.1016/j.cclet.2018.04.028
Abstract
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24
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The molecular assembling behaviours between ferrocene-modified diphenylalanine and
β
-cyclodextrin were investigated, which showed a reversible morphological conversion by the chemical redox of ferrocenyl moiety.
Supramolecular conducting microfibers from amphiphilic tetrathiafulvalene-based organogelator
Xuemei Liang, Lei Wang, Kwangun Jeong, Myonghoon Lee
CCL 2019 Vol. 30 (01): 123-126
DOI:10.1016/j.cclet.2018.07.001
Abstract
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23
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An amphiphilic tetrathiafulvalene molecule can gelate a variety of organic solvents in view of multiple intermolecular interactions, especially in polar solvent with the formation of highly-ordered columnar structures. The formation of mixed-valence states shows the semiconductive behaviors with the conductivity of 10
-4
S/cm, as promising candidates for organic electronics.
Self-assembly of supramolecular polymers in water from tetracationic and tetraanionic monomers in water through cooperative electrostatic attraction and aromatic stacking
Ya-Kun Zhao, Zhong-Zheng Gao, Hui Wang, Dan-Wei Zhang, Zhan-Ting Li
CCL 2019 Vol. 30 (01): 127-130
DOI:10.1016/j.cclet.2018.10.016
Abstract
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33
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The cooperative electrostatic attraction and
π-π
stacking between tetrahedral tetrapyridinium and three tetraanionic tetraphenylethylenes led to the formation of a new series of supramolecular polymers in water.
Facile construction of Zn(II)-porphyrin-cored [5]rotaxane and its controllable aggregation behaviours
Menglan He, Lijun Chen, Bo Jiang, Hongwei Tan, Cuihong Wang, Haibo Yang
CCL 2019 Vol. 30 (01): 131-134
DOI:10.1016/j.cclet.2018.10.035
Abstract
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31
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A novel Zn(Ⅱ)-porphorin-cored [5]rotaxane with platinum-acetylide as linkage was constructed. The obtained [5]rotaxane performed different morphologies in different solvents. In addition, the ordered morphologies generated from [5]rotaxane exhibited the morphology evolution by time.
To inhibit coffee ring effect in inkjet printing of light-emitting polymer films by decreasing capillary force
Xinhong Yu, Rubo Xing, Zhongxiang Peng, Yangming Lin, Zhonghui Du, Junqiao Ding, Lixiang Wang, Yanchun Han
CCL 2019 Vol. 30 (01): 135-138
DOI:10.1016/j.cclet.2018.09.007
Abstract
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27
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Coffee ring effects of inkjet printed poly(spirobifluorene) films were restrained by decreasing the capillary force due to volatility/viscosity match.
Handedness inversion of chiral mesoporous silica: A diffuse-reflectance circular dichroism study
Nan Wang, Ruiyu Lin, Minzhao Xue, Yingying Duan, Shun'ai Che
CCL 2019 Vol. 30 (01): 139-142
DOI:10.1016/j.cclet.2018.01.008
Abstract
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22
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Temperature-depended handedness inversion in chiral mesoporous silica was investigated by diffuse-reflectance circular dichroism spectra.
Effective enhancement of the emission efficiency of tetraphenylporphyrin in solid state by tetraphenylethene modification
Nan Jiang, Yijia Wang, Anjun Qin, Jing Zhi Sun, Ben Zhong Tang
CCL 2019 Vol. 30 (01): 143-148
DOI:10.1016/j.cclet.2018.10.020
Abstract
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20
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Evidently enhanced red emission efficiency from the solid state of tetraphenylporphyrin derivative was achieved by modification with tetraphenylethene units.
Creating super-tough and strong PA6/ABS blends using multi-phase compatibilizers
Xianwei Sui, Xu-Ming Xie
CCL 2019 Vol. 30 (01): 149-152
DOI:10.1016/j.cclet.2018.04.035
Abstract
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20
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PA6/ABS blends with excellent mechanical properties are prepared using combination of two effective multi-phase compatibilizers, where finely dispersed domains with unique encapsulation structures are generated for the synergistic improvement in tensile and impact performances.
Living and enantiomer-selective polymerization of allene initiated by Ni complex containing chiral phosphine
Hai Zhu, Shizhong Luo, Zongquan Wu
CCL 2019 Vol. 30 (01): 153-156
DOI:10.1016/j.cclet.2018.03.002
Abstract
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18
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In the polymerization of chiral allene by using chiral phosphine complex, the polymerization rate of L-
1
is approximately 1.9 times that of D-
1
. This catalyst has enantiomer-selectivity for the polymerization of chiral allene derivative monomer.
Coaxial electrospinning core-shell fibers for self-healing scratch on coatings
Pengchong Li, Zhi Shang, Kejian Cui, Huan Zhang, Zhi Qiao, Caizhen Zhu, Ning Zhao, Jian Xu
CCL 2019 Vol. 30 (01): 157-159
DOI:10.1016/j.cclet.2018.01.037
Abstract
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Polystyrene (PS) fibers with core-shell structure were prepared by coaxial electrostatic spinning using liquid epoxy or curing agent as the core and PS solution as the shell. Scratch self-healing coatings were realized by using the healant-loaded core-shell fibers in the matrix.
A novel
α
-fetoprotein-MIP immunosensor based on AuNPs/PTh modified glass carbon electrode
Yuxuan Lai, Chuanxiang Zhang, Yan Deng, Gaojian Yang, Song Li, Congli Tang, Nongyue He
CCL 2019 Vol. 30 (01): 160-162
DOI:10.1016/j.cclet.2018.07.011
Abstract
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A new alpha-fetoprotein-MIP (AFP-MIP) immunosensor based on glass carbon electrode (GCE) modified with polythionine (PTh) and gold nanoparticles (AuNPs) was successfully prepared for the sensitive detection of AFP. The AFP-MIP immunosensor presented a facile preparation, low sample consumption, and good stability, and could become a new promising method for the detection of AFP.
Nanoparticle structure transformation of mPEG grafted chitosan with rigid backbone induced by
α
-cyclodextrin
Lei Huang, Jiaojiao Chen, Muye He, Xinyu Hou, Yiben Lu, Kaiyan Lou, Feng Gao
CCL 2019 Vol. 30 (01): 163-166
DOI:10.1016/j.cclet.2017.12.012
Abstract
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22
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This paper presented an interesting nanoparticle-based drug-delivery system with morphology transition behavior depending on the content of exposed PEG chain on the particle surface and a likely mechanism for the morphological transition of the rod-coil graft copolymer mPEG-
g
-CS was proposed.
Preparation of Au nanoparticles modified TiO
2
nanotube array sensor and its application as chemical oxygen demand sensor
Longqi Liang, Jiao Yin, Jinpeng Bao, Linchuan Cong, Weimin Huang, Haibo Lin, Zhan Shi
CCL 2019 Vol. 30 (01): 167-170
DOI:10.1016/j.cclet.2018.01.049
Abstract
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Au nanoparticles (AuNPs) were electrodeposited at the highly ordered anatase TiO
2
nanotube array (TiO
2
NA) electrode to prepare the AuNP-TiO
2
NA sensor. The as-prepared sensor can be used for the determination of chemical oxygen demand (COD) in real samples.
Facile hydrothermal-thermal conversion synthesis of CaSiO
3
nanowires as promising structure and function integrated photoluminescent host candidate
Lin Xu, Panpan Sun, Xiuping Chen, Peiyan Zhai, Wancheng Zhu
CCL 2019 Vol. 30 (01): 171-174
DOI:10.1016/j.cclet.2018.03.001
Abstract
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A facile green hydrothermal-thermal conversion method was developed for the uniform high aspect ratio CaSiO
3
nanowires as promising structure and function integrated photoluminescent host, without any organic additive.
Controllable self-assembly of parallel gold nanorod clusters by DNA origami
Hang Yu, Tiantian Man, Wei Ji, Leilei Shi, Chenwei Wu, Hao Pei, Chuan Zhang
CCL 2019 Vol. 30 (01): 175-178
DOI:10.1016/j.cclet.2018.04.020
Abstract
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We demonstrate the self-assembly of three types of parallel gold nanorod clusters using a rod-like DNA origami as the template.
A multiple coupling approach to produce high-performance SERS substrates
Xianpeng Yin, Hao Dong, Shiqiang Wang, Yun Liang, Ning Gao, Wanlin Zhang, Li Tian, Fuwei Sun, Guangtao Li
CCL 2019 Vol. 30 (01): 179-182
DOI:10.1016/j.cclet.2018.06.013
Abstract
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In this work, large area gold-nanoparticle-cluster pillar array with a gold mirror as high-performance SERS substrate was facilely fabricated by combined use of nanosphere lithography and self-assembly approach.
Facile-fabricated iron oxide nanorods as a catalyst for hydrogenation of nitrobenzene
Yanshuang Ma, Liyun Zhang, Wen Shi, Yiming Niu, Bingsen Zhang, Dangsheng Su
CCL 2019 Vol. 30 (01): 183-186
DOI:10.1016/j.cclet.2018.04.034
Abstract
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Iron oxide nanorod catalysts were fabricated by wet chemistry method followed annealing. The facilefabricated FeOOH nanorods with an efficient catalytic performance for transfer hydrogenation of nitrobenzene with hydrazine hydrate are presented.
One-pot photoreduction to prepare NIR-absorbing plasmonic gold nanoparticles tethered by amphiphilic polypeptide copolymer for synergistic photothermal-chemotherapy
Siqi Yang, Linzhu Zhou, Yue Su, Rong Zhang, Chang-Ming Dong
CCL 2019 Vol. 30 (01): 187-191
DOI:10.1016/j.cclet.2018.02.015
Abstract
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We developed one-pot photoreduction strategy to fabricate the NIR-absorbing plasmonic PLC-
b
-PEO@Au NPs. It possessed strong NIR absorption at 700-1100 nm, an ultrahigh photothermal conversion efficiency of 62.1%, and good photostability.
Ultrafine molybdenum carbide nanoparticles supported on nitrogen doped carbon nanosheets for hydrogen evolution reaction
Kedong Xia, Junpo Guo, Cuijuan Xuan, Ting Huang, Zhiping Deng, Lingxuan Chen, Deli Wang
CCL 2019 Vol. 30 (01): 192-196
DOI:10.1016/j.cclet.2018.05.009
Abstract
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Nitrogen doped carbon nanosheets supported molybdenum carbides nanoparticles (Mo
x
C/NCS) have been synthesized by tuning the mass ratio of melamine and ammonia molybdate. The Mo
2
C/NCS-10 exhibits superior electrocatalytic performance and stability for HER, which was attributed to N-doped carbon nanosheets, small particle size, mesoporous structure, and large electrochemical active surface area.
MoS
2
decorated lignin-derived hierarchical mesoporous carbon hybrid nanospheres with exceptional Li-ion battery cycle stability
Feng Chen, Long Wu, Zeping Zhou, Jiajun Ju, Zhengping Zhao, Mingqiang Zhong, Tairong Kuang
CCL 2019 Vol. 30 (01): 197-202
DOI:10.1016/j.cclet.2018.10.007
Abstract
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We developed a feasible self-assembly and carbonization method to prepare lignin-derived porous carbon nanosphere (PCN) and its efficient embedment of MoS
2
without any additives. The obtained hybrid nanocomposite provides a possible route to develop high performance Li-ion battery from natural biomass or organizational structures.
Ethylenediamine promoted the hydrogenative coupling of nitroarenes over Ni/C catalyst
Youdi Yang, Shaopeng Li, Chao Xie, Hangyu Liu, Yanyan Wang, Qingqing Mei, Huizhen Liu, Buxing Han
CCL 2019 Vol. 30 (01): 203-206
DOI:10.1016/j.cclet.2018.04.006
Abstract
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In this work, we found that ethylenediamine can enrich the electron state of Ni and make the azobenzene easily desorb from the surface of the catalyst, which effectively inhibits the further hydrogenation to aniline and greatly improves the selectivity of azobenzene. When the ratio of Ni and ethylenediamine is 1:10, the yield of the azobenzene can reach 95.5%.
First-principles study of methanol adsorption on heteroatom-doped phosphorene
Dongdong Liu, Yongliang Shi, Li Tao, Dafeng Yan, Ru Chen, Shuangyin Wang
CCL 2019 Vol. 30 (01): 207-210
DOI:10.1016/j.cclet.2018.01.041
Abstract
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First-principles calculations were firstly employed to investigate the adsorption of methanol on pristine and X-doped phosphorene (X=B, C, N and O). The N and O doping improved the adsorption of phosphorene with CH
3
OH gas molecule, while B and C doping were almost not beneficial.
Electronic, optical, and charge transport properties of A-
π
-A electron acceptors for organic solar cells: Impact of anti-aromatic
π
structures
Yan Zeng, Ruihong Duan, Yuan Guo, Guangchao Han, Qingxu Li, Yuanping Yi
CCL 2019 Vol. 30 (01): 211-216
DOI:10.1016/j.cclet.2018.05.029
Abstract
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22
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Anti-aromatization and isomerization are found to be an effective way to tune the optoelectronic properties of A-
π
-A electron acceptors for organic photovoltaics.
Effects of processing additives in non-fullerene organic bulk heterojunction solar cells with efficiency >11%
Shenkun Xie, Jianqiu Wang, Rong Wang, Dongyang Zhang, Huiqiong Zhou, Yuan Zhang, Defeng Zhou
CCL 2019 Vol. 30 (01): 217-221
DOI:10.1016/j.cclet.2018.04.001
Abstract
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17
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The solar cell surface morphologies with different additives observed with slightly changed in roughness. It is easily to get the best PCE of 11.1% with using 0.5% DIO additives.
Simple non-fullerene electron acceptors with unfused core for organic solar cells
Yao Li, Yunhua Xu, Fan Yang, Xudong Jiang, Cheng Li, Shengyong You, Weiwei Li
CCL 2019 Vol. 30 (01): 222-224
DOI:10.1016/j.cclet.2018.09.014
Abstract
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21
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Two simple unfused-cores based electron acceptors with different side units were developed for application in non-fullerene solar cells, in which the side chains have the significant effect on their absorption spectra and photovoltaic performance.
Photocatalytic hydrogen production from acidic aqueous solution in BODIPY-cobaloxime-ascorbic acid homogeneous system
An Xie, Zhong-Hua Pan, Miao Yu, Geng-Geng Luo, Di Sun
CCL 2019 Vol. 30 (01): 225-228
DOI:10.1016/j.cclet.2018.05.003
Abstract
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24
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For the first time, iodinated BODIPY dyes with phenylamine or 8-hydroxylquinoline moiety at the
meso
-position on the BODIPY core were tested for the light-driven production of H
2
from the acidic aqueous solutions.
Co
1-x
S embedded in porous carbon derived from metal organic framework as a highly efficient electrocatalyst for oxygen evolution reaction
Denghong He, Xiaolin Wu, Wei Liu, Chaojun Lei, Chunlin Yu, Guokui Zheng, Junjie Pan, Lecheng Lei, Xingwang Zhang
CCL 2019 Vol. 30 (01): 229-233
DOI:10.1016/j.cclet.2018.03.020
Abstract
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24
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Here, we report a two-step conversion method to fabricate a composite of Co
1-x
S embedded in porous carbon framework (Co
1-x
S@C) derived from metal organic frameworks (MOFs). The as-prepared porous dodecahedron Co
1-x
S@C composite catalyst exhibits excellent electrocatalytic performance towards oxygen evolution reaction (OER).
An anionic In(III)-based metal-organic framework with Lewis basic sites for the selective adsorption and separation of organic cationic dyes
Qi Yang, Bin Wang, Ya Chen, Yabo Xie, Jianrong Li
CCL 2019 Vol. 30 (01): 234-238
DOI:10.1016/j.cclet.2018.03.023
Abstract
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25
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An In(Ⅲ)-based metal-organic framework (
BUT-29
) can selectively absorb cationic dyes in DMF even in the presence of other organic dyes, and has the higher adsorption capacity.
Biologically inspired silk fibroin grafted polyacrylonitrile filtration membrane prepared in ZnCl
2
aqueous solution
Jingang Li, Shuwen Li, Xiaohui Wang, Fan Fan, Kongyin Zhao, Junfu Wei, Linhua Zhang, Dunwan Zhu
CCL 2019 Vol. 30 (01): 239-242
DOI:10.1016/j.cclet.2018.07.016
Abstract
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23
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Biologically inspired silk fibroin grafted polyacrylonitrile (SF-
g
-PAN) filtration membrane was prepared using ZnCl
2
aqueous solution as solvent, avoiding the use of organic solvents.
Design, synthesis and biological evaluation of a novel platinum(II) complex possessing bioreductive groups for cancer therapy
Chengken Chen, Chunmei Gao, Zigao Yuan, Yuyang Jiang
CCL 2019 Vol. 30 (01): 243-246
DOI:10.1016/j.cclet.2018.04.010
Abstract
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28
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A Pt(Ⅱ) complex possessing bioreductive groups was constructed and evaluated as a more potent antitumor agent than cisplatin.
Design and synthesis of novel water-soluble amino acid derivatives of chlorin p6 ethers as photosensitizer
Xingjie Zhang, Zhi Meng, Zhiqiang Ma, Junhong Liu, Guiyan Han, Fujia Ma, Ningyang Jia, Zhenyuan Miao, Wannian Zhang, Chunquan Sheng, Jianzhong Yao
CCL 2019 Vol. 30 (01): 247-249
DOI:10.1016/j.cclet.2018.04.029
Abstract
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17
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Eight new water-soluble amino acid derivatives of chlorin p
6
ethers
6a-h
were designed and synthesized using purpurin-18 (
2
) as key intermediate. All target compounds exhibited better phototoxicity than talaporfin and the most phototoxic compound
6d
showed IC
50
values of 0.20 μmol/L against A549 cell and 0.41 μmol/L against B16-F10 cell, which represented 31- and 24-fold increase of PDT antitumor efficacy compared to talaporfin.
Novel dual inhibitors against FP-2 and PfDHFR as potential antimalarial agents: Design, synthesis and biological evaluation
Wenhua Chen, Xue Yao, Zhenghui Huang, Fei Mao, Longfei Guan, Yun Tang, Hualiang Jiang, Jian Li, Jin Huang, Lubin Jiang, Jin Zhu
CCL 2019 Vol. 30 (01): 250-254
DOI:10.1016/j.cclet.2017.11.041
Abstract
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23
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A series of novel 2,4-diaminopyrimidine-modified compounds was designed and synthesized. Compound
14
showed micromolar dual inhibitory effect on both FP-2 and PfDHFR, and potential inhibition to the proliferation of
P. falciparum
3D7 strain and chloroquine-resistant
P. falciparum
Dd2 strain.
Water bridges are essential to neonicotinoids: Insights from synthesis, bioassay and molecular modelling studies
Chengchun Zhu, Guanglong Li, Keya Xiao, Xusheng Shao, Jiagao Cheng, Zhong Li
CCL 2019 Vol. 30 (01): 255-258
DOI:10.1016/j.cclet.2018.05.013
Abstract
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20
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To identify the detailed roles of water bridges in neonicotinoids recognition, twenty-four neonicotinoids compounds were designed, synthesized, bioassayed and modelled. Of all nine fragments mimicking water bridges, cyano group was the optimal one. The insecticidal activities indicated that the water bridge might be stable in the active site and was not suitable to be replaced by other groups, which highlighted the significance of water bridges for neonicotinoids.
Tetra-phthalimide end-fused bifluorenylidene: Synthesis and characterization
Debin Xia, Fangyuan Zhang, Zhigang Liu, Linghao Meng, Ruiqing Fan, Yulin Yang
CCL 2019 Vol. 30 (01): 259-262
DOI:10.1016/j.cclet.2018.01.033
Abstract
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A novel electron acceptor, namely, tetra-phthalimide end-fused bifluorenylidene (3D-imide) was designed and synthesized.
Gram-scale preparation of dialkylideneacetones through Ca(OH)
2
-catalyzed Claisen-Schmidt condensation in dilute aqueous EtOH
Hao Zhang, Mengting Han, Chenggen Yang, Lei Yu, Qing Xu
CCL 2019 Vol. 30 (01): 263-265
DOI:10.1016/j.cclet.2018.01.035
Abstract
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22
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A practical synthetic method of dialkylideneacetones has been developed. Compared with known protocols, the method employed catalytic Ca(OH)
2
as the cheap, mild base catalyst and dilute aqueous EtOH (20%, v/v) as the green and safe solvent. The products could be synthesized in gram-scale and isolated by a simple filtration.
One-pot synthesis of tetrahydroindoles
via
a copper catalyzed
N
-alkynation/[4+2] cycloaddition cascade
Chun Jiang, Piao-Piao Yu, Qing Zhang, Hua-Dong Xu, Mei-Hua Shen
CCL 2019 Vol. 30 (01): 266-268
DOI:10.1016/j.cclet.2018.05.040
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4,7-Dihydroindolines are prepared from alkyne bromides and 2-dienyl sulfonamides
via
a CuSO
4
catalyzed cascade in a one-pot fashion.
A one-pot protocol for copper-mediated azide-alkyne cycloaddition using alkenyl triflate precursors
Yu Chen, Lianchao Liu, Dimin Wu, Yu-Peng He, Ang Li
CCL 2019 Vol. 30 (01): 269-270
DOI:10.1016/j.cclet.2018.06.001
Abstract
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Taking advantage of LiCl-promoted elimination of alkenyl triflates, we developed a one-pot protocol for copper-mediated azide-alkyne cycloaddition using alkenyl triflate precursors, which may find potential use in sequential click reactions.
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